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Please use this identifier to cite or link to this item: http://hdl.handle.net/10016/6947

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Title: Dynamics of rough interfaces in Chemical Vapor Deposition: experiments and model for silica films
Author(s): Ojeda, Fernando
Cuerno, Rodolfo
Salvarezza, Roberto
Vázquez, Luis
Publisher: The American Physical Society
Issued date: 3-Apr-2000
Citation: Physical Review Letters, 2000, vol. 84, n. 14, p. 3125-3128
URI: http://hdl.handle.net/10016/6947
ISSN: 0031-9007 (Print)
1079-7114 (Online)
DOI: 10.1103/PhysRevLett.84.3125
Description: 4 pages, 5 figures.-- PACS nrs.: 68.55.Jk, 05.10.Gg, 64.60.Ht, 81.15.Gh.-- ArXiv pre-print available at: http://arxiv.org/abs/cond-mat/0003155
Final publisher version available Open Access at: http://gisc.uc3m.es/~cuerno/publ_list.html
Abstract: We study the surface dynamics of silica films grown by low pressure chemical vapor deposition. Atomic force microscopy measurements show that the surface reaches a scale invariant stationary state compatible with the Kardar-Parisi-Zhang (KPZ) equation in three dimensions. At intermediate times the surface undergoes an unstable transient due to shadowing effects. By varying growth conditions and using spectroscopic techniques, we determine the physical origin of KPZ scaling to be a low value of the surface sticking probability, related to the surface concentration of reactive groups. We propose a stochastic equation that describes the qualitative behavior of our experimental system.
Sponsor: This work has been performed within the CONICET-CSIC and Programa de Cooperación con Iberoamérica (MEC) research programs, and has been partially supported by CAM Grants No. 7220-ED/082, No. 07N-0028, and DGES Grants No. MAT97-0698-C04 and No. PB96-0119. F. O. acknowledges support by CAM.
Review: PeerReviewed
Publisher version: http://dx.doi.org/10.1103/PhysRevLett.84.3125
Keywords: [PACS] Structure and morphology; thickness; crystalline orientation and texture
[PACS] Stochastic analysis methods (Fokker-Planck, Langevin, etc.)
[PACS] Dynamic critical phenomena
[PACS] Chemical vapor deposition (including plasma-enhanced CVD, MOCVD, ALD, etc.)
Rights: © The American Physical Society
Appears in Collections:DM - GISC - Artículos de Revistas

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